四川盆地南缘筠连乐平组煤层气地球化学特征及多源富集模式

Geochemical characterization of coalbed methane in Leping Formation and its multi-source enrichment pattern in Junlian, southern Sichuan Basin

  • 摘要: 四川盆地南缘筠连煤层气区块是南方第1个成功开发的商业性区块,煤层气井具有“日均产量高、累计产量高、稳产期长”的产出特征,然而煤储层具有“高灰分、高含气量、高含气饱和度”的异常特殊性。为揭示川南筠连区块气体成因以及来源,以29口煤层气井产出气和4口煤矿煤样为研究对象,开展了煤岩学、碳同位素、流体包裹体、产出气组分、碳氢同位素试验,结合区域构造演化与盆地模拟结果,系统揭示了研究区煤层气的成因类型、气体来源与运移规律,建立了本区煤层气富集成藏模式。结果表明:乐平组煤岩碳同位素比值平均为−23.1‰,显微组分以镜质组为主,其次为惰质组,不含壳质组,烃源岩主要为III型(腐植型)干酪根。产出气组分以CH4为主,重烃含量极低,属于极干性气体,δ13C1值平均为−34.1‰,δ13C2值平均为−31.2‰,表现为正碳同位素组成序列,δD1值平均为−131.3‰。产出气为高−过成熟阶段的热成因气,气体类型为油型气,烃源岩为腐泥型干酪根,与煤系地层为腐植型干酪根的结论不符。结合研究区地质背景,通过区域气源对比,认为上二叠统乐平组产出气为自生自储式煤层气与下生上储式页岩气的混合气。显微裂隙交叉切割关系、包裹体定向排列方向以及均一温度的双峰特征表明煤层气成藏过程分为2期,分别为早白垩世生烃高峰期和晚白垩世构造抬升期。盆地模拟结果显示,龙马溪组页岩气在燕山期抬升过程中沿断层向上运移,被乐平组煤层捕获,形成“下生上储”式混合气藏,煤层高含气量得益于页岩气补充及煤系地层较强的封存能力。

     

    Abstract: Junlian coalbed methane (CBM) block at the southern edge of Sichuan Basin is the first successfully developed commercial block in the south, and the CBM wells have the output characteristics of “high average daily production, high cumulative production, and long stable production period”, but the coal reservoirs have the anomalous special characteristics of “high ash content, high gas content, and high gas saturation”. To investigate the origin and source of gas in the Junlian Block of southern Sichuan, a study was conducted using gas produced from 29 CBM wells and coal samples from 4 coal mines as research objects. The study involved coal petrology, carbon isotope analysis, fluid inclusion analysis, gas composition analysis, and carbon-hydrogen isotope experiments. Combined with regional tectonic evolution and basin simulation results, the study systematically revealed the genesis types, gas sources, and migration patterns of CBM in the study area, and established a CBM accumulation model for the region. The results show that: the average carbon isotope value of coal rocks in the Leping Formation is −23.1‰, the maceral group is dominated by the vitrinite, followed by the inertinite, without the liptinite, and the hydrocarbon source rock is mainly the type III (humic) kerogen. The output gas component is dominated by CH4, with very low heavy hydrocarbon content, and belongs to extremely dry gas, with δ13C1 averaging −34.1‰ and δ13C2 averaging −31.2‰, which manifests positive carbon isotope composition sequence, and the δD1 value averaging −131.3‰. The output gas is thermogenic gas of high-over-mature stage, the gas type is oil-type gas, and the hydrocarbon source rock is sapropelic kerogen, which is inconsistent with the conclusion that the coal stratum is humic kerogen. Combined with the geological background of the study area, through the comparisons of regional gas-source rock, it is believed that the gas produced from Upper Permian Leping Formation is a mixture of self-generated and self-stored CBM and downgraded and upgraded shale gas. The microfracture cross-cutting relationship, the oriented alignment direction of inclusions and the bimodal characteristics of homogeneous temperature indicate that the CBM formation process is divided into two phases, namely the Early Cretaceous hydrocarbon peak and the Late Cretaceous tectonic uplift. Basin simulation results show that Longmaxi Formation shale gas was transported upward along the faults during Yanshanian period uplift, and was captured by the coal beds of Leping Formation, forming a mixed gas reservoir of the “down-generation and up-storage” type, and the high gas content in the coal beds is attributed to the supplementation of the shale gas and the strong sealing ability of the coal strata.

     

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